The PSU's in both computers, that this HDD has been connected to, both seem to be sound. In the main unRaid unit (using a Corsair TX650W PSU) there are 11 other HDD's that seem to be free of the issues that this one has. In terms of vibration, when it was a part of the main array it was secured using silicone grommets. As you suggest, I will RMA, but include a note mentioning the continual sectors pending re-allocation.
Thanks again for the assistance.
Cheers