@trurl Thanks again. After further review, based on the articles you sent, I wanted to provide some updates.
Shares - I reviewed the shares and have reasons for why everything is configured the way it is. Specifically, what's pinned to cache is setup for speed of processing particular functions. It was good to review all the same, but I wanted you to know that it's configured as intended.
Memory - Based on the article you linked above, and with the help of a friend, I started digging into my memory. What we found was that one of the 4 DIMMs was not being recognized in the BIOS and Unraid. I'm not sure how or when this DIMM went missing from the system, but after reseating all 4 of them, they all came back online. I'm hopeful that this was the culprit and your article above is what put me on this path, so THANK YOU!
Overclock - I am overclocking the memory beyond what is supported (again thank you for the linked thread), but I've been running in this state for over 2 years with no issues until somewhat recently. Should the crashing persist, I'll drop the mem to the specs outlined per support.
I'll follow-up to let you know if the server remains stable after resolving the missing DIMM issue and if not, I'll provide additional specifics.
Thank you again!