According to these latest diagnostics:
b-----s shareUseCache="no" # Share exists on disk1
b--------n shareUseCache="only" # Share exists on disk1
isos shareUseCache="only" # Share exists on disk1
M--------a shareUseCache="yes" # Share exists on cache, disk1
system shareUseCache="only" # Share exists on cache, disk1
T---------e shareUseCache="only" # Share exists on disk1
u------p shareUseCache="only" # Share exists on cache, disk1
So, you have several shares set to only use the cache drive, but they have files on disk1, including the earlier mentioned "system" share.
Merely changing the settings will not move anything. In fact, changing a share to only use cache will guarantee that mover will ignore it, since it is not possible to set a Mover action for shares without Secondary storage.
Also, syslog has several entries where mover says the file already exists. Mover won't replace files.
And nothing can move or delete open files, so you have to disable Docker and VM Manager in Settings to work with some of these.
Might be simpler to clean this up yourself using Dynamix File Manager.